Tuesday, July 5, 2011

3,7-Diazadibenzophosphole Oxide: A Phosphorus-Bridged Viologen Analogue with Significantly Lowered Reduction Threshold

3,7-Diazadibenzophosphole Oxide: A Phosphorus-Bridged Viologen Analogue with Significantly Lowered Reduction Threshold: "
Thumbnail image of graphical abstract

Phosphorus pulls its weight: Installation of a phosphoryl group as central bridge in the 4,4′-bipyridine scaffold introduces improved reduction responses that become even more pronounced in the corresponding phosphoryl-bridged methylviologen (see picture). Importantly, the scaffold maintains the typical viologen optical response upon reversible reduction, however, at much lower potentials.

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